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Highly permeable artificial water channels that can self-assemble into two-dimensional arrays 期刊论文

编号：

7d5adfb2-9b13-45bd-9035-03cdeb495cf7
作者：

Shen, Yuexiao^[1] Si, Wen^[2] Erbakan, Mustafa^[1] Decker, Karl^[3] De Zorzi, Rita^[4,5] Saboe, Patrick O.^[1] Kang, You Jung^[6] Majd, Sheereen^[6] Butler, Peter J.^[6] Walz, Thomas^[4,5] Aksimentiev, Aleksei^[3] Houb, Junli^[2] Kumar, Manish^[1]
语种：

English
期刊：

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA ISSN：0027-8424 2015 年 112 卷 32 期 (9810 - 9815) ; AUG 11
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关键词：

artificial aquaporins artificial water channels peptide-appended pillar[5]arene single-channel water permeability two-dimensional arrays
摘要：

Bioinspired artificial water channels aim to combine the high permeability and selectivity of biological aquaporin (AQP) water channels with chemical stability. Here, we carefully characterized a class of artificial water channels, peptide-appended pillar[5]arenes (PAPs). The average single-channel osmotic water permeability for PAPs is 1.0(+/- 0.3) x 10(-14) cm(3)/s or 3.5(+/- 1.0) x 10(8) water molecules per s, which is in the range of AQPs (3.4 similar to 40.3 x 10(8) water molecules per s) and their current synthetic analogs, carbon nanotubes (CNTs, 9.0 x 10(8) water molecules per s). This permeability is an order of magnitude higher than first-generation artificial water channels (20 to similar to 10(7) water molecules per s). Furthermore, within lipid bilayers, PAP channels can self-assemble into 2D arrays. Relevant to permeable membrane design, the pore density of PAP channel arrays (similar to 2.6 x 10(5) pores per mu m(2)) is two orders of magnitude higher than that of CNT membranes (0.1 similar to 2.5 x 10(3) pores per mu m(2)). PAP channels thus combine the advantages of biological channels and CNTs and improve upon them through their relatively simple synthesis, chemical stability, and propensity to form arrays.
推荐引用方式
GB/T 7714：

Shen Yue-xiao,Si Wen,Erbakan Mustafa, et al. Highly permeable artificial water channels that can self-assemble into two-dimensional arrays [J].PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,2015,112(32):9810-9815.
APA：

Shen Yue-xiao,Si Wen,Erbakan Mustafa,Decker Karl,&Kumar Manish.(2015).Highly permeable artificial water channels that can self-assemble into two-dimensional arrays .PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,112(32):9810-9815.
MLA：

Shen Yue-xiao, et al. "Highly permeable artificial water channels that can self-assemble into two-dimensional arrays" .PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA 112,32(2015):9810-9815.

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