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Human exposure to PCDDs and their precursors from heron and tern eggs in the Yangtze River Delta indicate PCP origin 期刊论文

编号：

a619ee7d-935f-42b3-b1c3-18b5979d4e3c
作者：

Zhou, Yihui^[1,2] Yin, Ge^[2] Asplund, Lillemor^[2] Stewart, Kathryn^[1] Rantakokko, Panu^[3] Bignert, Anders^[4,5] Ruokojarvi, Paivi^[3] Kiviranta, Hannu^[3] Qiu, Yanling^[5] Ma, Zhijun^[6] Bergman, Ake^[1,2,7]
语种：

英文
期刊：

ENVIRONMENTAL POLLUTION ISSN：0269-7491 2017 年 225 卷 (184 - 192) ; JUN
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关键词：

PCDD/Fs PCDEs PCP OH-PCDEs Yangtze river delta Bird egg
摘要：

Polychlorinated dibenzo-p-dioxins (PCDDs) and polychlorinated dibenzofurans (PCDFs) are highly toxic to humans and wildlife. In the present study, PCDD/Fs were analyzed in the eggs of whiskered terns (Chlidonias hybrida), and genetically identified eggs from black-crowned night herons (Nycticorax nycticorax) sampled from two lakes in the Yangtze River Delta area, China. The median toxic equivalent (TEQ) of PCDD/Fs were 280 (range: 95-1500) and 400 (range: 220-1100) pg TEQ g(-1) lw (WHO, 1998 for birds) in the eggs of black-crowned night heron and whiskered tern, respectively.
Compared to known sources, concentrations of PCDDs relative to the sum of PCDD/Fs in bird eggs, demonstrated high abundance of octachlorodibenzo-p-dioxin (OCDD), 1,2,3,4,6,7,8-heptaCDD and 1,2,3,6,7,8-hexaCDD indicating pentachlorophenol (PCP), and/or sodium pentachlorophenolate (Na-PCP) as significant sources of the PCDD/Fs. The presence of polychlorinated diphenyl ethers (PCDEs), hydroxylated and methoxylated polychlorinated diphenyl ethers (OH-and Me0-PCDEs, known impurities in PCP products), corroborates this hypothesis. Further, significant correlations were found between the predominant congener CDE-206, 3'-OH-CDE-207, 2'-MeO-CDE-206 and OCDD, indicating a common origin.
Eggs from the two lakes are sometimes used for human consumption. The WHO health-based tolerable intake of PCDD/Fs is exceeded if eggs from the two lakes are consumed regularly on a weekly basis, particularly for children. The TEQs extensively exceed maximum levels for PCDD/Fs in hen eggs and egg products according to EU legislation (2.5 pg TEQ g(-1)/w). The results suggest immediate action should be taken to manage the contamination, and further studies evaluating the impacts of egg consumption from wild birds in China. Likewise, studies on dioxins and other POPs in common eggs need to be initiated around China. (C) 2017 The Authors. Published by Elsevier Ltd.
推荐引用方式
GB/T 7714：

Zhou Yihui,Yin Ge,Asplund Lillemor, et al. Human exposure to PCDDs and their precursors from heron and tern eggs in the Yangtze River Delta indicate PCP origin [J].ENVIRONMENTAL POLLUTION,2017,225:184-192.
APA：

Zhou Yihui,Yin Ge,Asplund Lillemor,Stewart Kathryn,&Bergman Ake.(2017).Human exposure to PCDDs and their precursors from heron and tern eggs in the Yangtze River Delta indicate PCP origin .ENVIRONMENTAL POLLUTION,225:184-192.
MLA：

Zhou Yihui, et al. "Human exposure to PCDDs and their precursors from heron and tern eggs in the Yangtze River Delta indicate PCP origin" .ENVIRONMENTAL POLLUTION 225(2017):184-192.

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